Friday, September 16, 2022

3D quantum spin liquid discovery gains theoretical support

Amazing stuff! Exotic physics or is there more to it?

"... Then, in 2019, researchers ... found experimental evidence that a pyrochlore magnet, Ce2Zr2O7, could be a long-sought-after example of a three-dimensional quantum spin liquid (3D QSL). This “experimental conjecture” has now received further support from physicists ... the researchers used a combination of theoretical techniques to conclude that Ce2Zr2O7 (CZO for short) is indeed a 3D QSL. ...
QSL will remain in a liquid state even at temperatures near absolute zero, where most materials freeze solid. ..."

From the abstract:
"The search for quantum spin liquids—topological magnets with fractionalized excitations—has been a central theme in condensed matter and materials physics. Despite numerous theoretical proposals, connecting experiment with detailed theory exhibiting a robust quantum spin liquid has remained a central challenge. Here, focusing on the strongly spin-orbit coupled effective S = 1/2 pyrochlore magnet Ce2Zr2O7, we analyze recent thermodynamic and neutron-scattering experiments, to identify a microscopic effective Hamiltonian through a combination of finite temperature Lanczos, Monte Carlo, and analytical spin dynamics calculations. Its parameter values suggest the existence of an exotic phase, a π-flux U(1) quantum spin liquid. Intriguingly, the octupolar nature of the moments makes them less prone to be affected by magnetic disorder, while also hiding some otherwise characteristic signatures from neutrons, making this spin liquid arguably more stable than its more conventional counterparts."

3D quantum spin liquid discovery gains theoretical support – Physics World


Fig. 1: Quantum spin liquid in a pyrochlore magnet and its experimental ramifications


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